We use 365 at work with one drive. We have our files on our pc but then take the folders we work on the most and copy them into one drive. Now every time we add another file our the folders on our work pc it copies them into the one drive folder as well. We also have a shared one drive folder that everyone can access within the company. Doing this allows us to access the folders on our phones or personal pc's at home should we want to or need to work remotly.
Also vouching for one drive however I'm using it on my Mac.
One thing you can do in Onedrive on a Mac is 'mimic' the standard directory structure within the one drive (sync/backed up folder), adfter which you can update all the quick access folders etc in the finder winder to point to one driver folders but essentisally it looks as if you're just working on a standard Mac setup using its SSD.
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